Which nuclear data can be validated with LLNL pulsed-sphere experiments?

It is shown here that 14-MeV D+T LLNL pulsed-sphere experiments bring complementary information into the process of validating nuclear data compared to experiments that are traditionally used for this purpose?such as critical assemblies. To be more specific, the 14-MeV D+T LLNL pulsed-sphere neutron-leakage spectra enable to validate scattering and fission nuclear data up to 15 MeV (compared to approximately up to 5 MeV when using criticality experiments) and employ to this end simple compound targets containing only few isotopes. Sensitivity profiles of the spectra to nuclear data are calculated in order to understand in detail which isotopes, observables, and energy ranges of nuclear data contribute significantly to their simulation. These profiles are presented for a few selected spheres containing ¹⁶O, ¹²C, ⁵⁶Fe, and ²³⁹Pu. It is shown that the neutron-leakage spectra of spheres containing light elements are mostly sensitive to elastic- and inelastic-scattering cross sections on discrete levels and corresponding angular distributions. Spheres of structural materials are sensitive to elastic- and inelastic scattering cross sections, including scattering on discrete levels and the continuum, and double differential cross sections. Actinide spheres are also strongly sensitive to the fission observables, in particular to the total-fission neutron spectrum. Thin spheres (in which neutrons experience on average less than one scatter) are mostly sensitive to data near the elastic peak, in the energy range from 12-15 MeV, while thicker ones can be sensitive to data at lower incident-neutron energies due to multiple-scattering effects. This information is brought together with simulations of 71 pulsed-sphere neutron-leakage spectra using the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear-data libraries. This analysis highlights ENDF/BVIII. 0 data that could be further investigated for potential shortcomings (⁶Li, ¹²C, ¹⁶O, ^24-26Mg, ²⁷Al, ⁴⁸Ti, ⁵⁶Fe, and ²⁰⁸Pb) or are likely reliable (^1,2H, ⁷Li, ⁹Be, ¹⁴N, ^235,238U, and ²³⁹Pu) as indicated by validating with LLNL pulsed-sphere experiments.