Published 2014
NDS Staff Publication
Zirconium evaluations for ENDF/B-VII.2 for the fast region
- 1. Nuclear Data Section, IAEA
Description
We have performed a new combined set of evaluations for 90−96Zr, including new resolved resonance
parameterizations from Said Mughabghab for 90,91,92,94,96Zr and fast region calculations
made with EMPIRE-3.1. Because 90Zr is a magic nucleus, stable Zr isotopes are nearly spherical.
A new soft-rotor optical model potential is used allowing calculations of the inelastic scattering on
low-lying coupled levels of vibrational nature. A soft rotor model describes dynamical deformations
of the nucleus around the spherical shape and is implemented in EMPIRE/OPTMAN code. The
same potential is used with rigid rotor couplings for odd-A nuclei. This then led to improved elastic
angular distributions, helping to resolve improper leakage in the older ENDF/B-VII.1β evaluation
in KAPL proprietary, ZPR and TRIGA benchmarks. Another consequence of 90Zr being a magic
nucleus is that the level densities in both 90Zr and 91Zr are unusually low causing the (n,el) and
(n,tot) cross sections to exhibit large fluctuations above the resolved resonance region. To accommodate
these fluctuations, we performed a simultaneous constrained generalized least-square fit to
(n,tot) for all isotopic and elemental Zr data in EXFOR, using EMPIRE's TOTRED scaling factor.
TOTRED rescales total cross sections so that the optical model calculations are unaltered by the
rescaling and the correct competition between channels is maintained. In this fit, all (n,tot) data
in EXFOR was used for Ein > 100 keV, provided the target isotopic makeup could be correctly
understood, including spectrum averaged data and data with broad energy resolution. As a result
of our fitting procedure, we will have full cross material and cross reaction covariance for all Zr
isotopes and reactions.